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Luckily, the actress rebounded with a performance thought by many critics to be the best of her career, when she re-teamed with one of her earliest champions, Pedro Almodóvar, for his nostalgic, bittersweet Volver in 2006.
She was nominated the next year for the Golden Globe, the Screen Actors Guild, and the Oscar for her sexy supporting turn in Rob Marshall's big-screen adaptation of the hit Broadway musical Nine.
Despite the film itself doing poorly, Cruz proved that she'd found a solid career trajectory as the 2010's progressed, appearing in projects like Pirates of the Caribbean: On Stranger Tides.
In 1998, Cruz had her first starring role in an English-language film, playing Billy Crudup's Mexican-American love interest in Stephen Frears' The Hi-Lo Country.
She had another go at English later that year in the Spanish-British romantic comedy Twice Upon a Yesterday, which cast her as a Spanish barmaid living in London.
The former cast her as the desperately poor daughter of a village prostitute, while the latter featured her as one of four lusty daughters of a wealthy man in pre-Franco Spain.
Belle Epoque proved to be a huge success, winning nine Goya Awards (the Spanish equivalent of an Academy Award) and an Oscar for Best Foreign Film.
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Gaining notice for her roles in All the Pretty Horses in 2000 and Blow the following year, it appeared as if Cruz's career had suddenly kicked into overdrive.
After starring alongside Nicolas Cage in the underperforming Captain Corelli's Mandolin in 2001, Cruz dove back into familiar territory with director Cameron Crowe's remake of Abre los Ojos, Vanilla Sky (2001).
Developing a close relationship with lead Tom Cruise as his much publicized breakup with Nicole Kidman drew to a close, the pair soon found themselves the center of considerable paparazzi attention as they became Hollywood's hottest new couple.